138 research outputs found
Effects of Fe doping in La1/2Ca1/2MnO3
The effect of Fe doping in the Mn site on the magnetic, transport and
structural properties of polycrystalline La1/2Ca1/2MnO3 was studied. Doping
with low Fe concentration (< 10%) strongly affects electrical transport and
magnetization. Long range charge order is disrupted even for the lowest doping
level studied (~2%). For Fe concentration up to 5% a ferromagnetic state
develops at low temperature with metallic like conduction and thermal
hysteresis. In this range, the Curie temperature decreases monotonously as a
function of Fe doping. Insulating behavior and a sudden depression of the
ferromagnetic state is observed by further Fe doping.Comment: 2 pages, presented at ICM2000, to appear in JMM
Critical structure factor in Ising systems
We perform a large-scale Monte Carlo simulation of the three-dimensional
Ising model on simple cubic lattices of size L^3 with L=128 and 256. We
determine the corresponding structure factor (Fourier transform of the
two-point function) and compare it with several approximations and with
experimental results. We also compute the turbidity as a function of the
momentum of the incoming radiation, focusing in particular on the deviations
from the Ornstein-Zernicke expression of Puglielli and Ford.Comment: 16 page
Kitaev interactions in the Co honeycomb antiferromagnets Na3Co2SbO6 and Na2Co2TeO6
Co ions in an octahedral crystal field, stabilise a j = 1/2
ground state with an orbital degree of freedom and have been recently put
forward for realising Kitaev interactions, a prediction we have tested by
investigating spin dynamics in two cobalt honeycomb lattice compounds,
NaCoTeO and NaCoSbO, using inelastic neutron
scattering. We used linear spin wave theory to show that the magnetic spectra
can be reproduced with a spin Hamiltonian including a dominant Kitaev
nearest-neighbour interaction, weaker Heisenberg interactions up to the third
neighbour and bond-dependent off-diagonal exchange interactions. Beyond the
Kitaev interaction that alone would induce a quantum spin liquid state, the
presence of these additional couplings is responsible for the zigzag-type
long-range magnetic ordering observed at low temperature in both compounds.
These results provide evidence for the realization of Kitaev-type coupling in
cobalt-based materials, despite hosting a weaker spin-orbit coupling than their
4d and 5d counterparts
Magnetisation Studies of Geometrically Frustrated Antiferromagnets SrLn2O4, with Ln = Er, Dy and Ho
We present the results of susceptibility \chi(T) and magnetisation M(H)
measurements performed on single crystal samples of the rare-earth oxides
SrLn2O4 (Ln = Er, Dy and Ho). The measurements reveal the presence of magnetic
ordering transition in SrHo2O4 at 0.62 K and confirm that SrEr2O4 orders
magnetically at 0.73 K, while in SrDy2O4 such a transition is absent down to at
least 0.5 K. The observed ordering temperatures are significantly lower than
the Curie-Weiss temperatures, \theta_{CW}, obtained from the high-temperature
linear fits to the 1/\chi(T) curves, which implies that these materials are
subject to geometric frustration. Strong anisotropy found in the \chi(T) curves
for a field applied along the different crystallographic directions is also
evident in the M(H) curves measured both above and below the ordering
temperatures. For all three compounds the magnetisation plateaux at
approximately one third of the magnetisation saturation values can be seen for
certain directions of applied field, which is indicative of field-induced
stabilisation of a collinear {\it two-up one-down} structure.Comment: 6 pages, 6 figure
Phase Competition in Ln0.5a0.5mno3 Perovskites
Single crystals of the systems Pr0.5(Ca1-xSrx)0.5MnO3,
(Pr1-yYy)0.5(Ca1-xSrx)0.5MnO3, and Sm0.5Sr0.5MnO3 were grown to provide a
series of samples with fixed ratio Mn(III)/Mn(IV)=1 having geometric tolerance
factors that span the transition from localized to itinerant electronic
behavior of the MnO3 array. A unique ferromagnetic phase appears at the
critical tolerance factor tc= 0.975 that separates charge ordering and
localized-electron behavior for t<tc from itinerant or molecular-orbital
behavior for t>tc. This ferromagnetic phase, which has to be distinguished from
the ferromagnetic metallic phase stabilized at tolerance factors t>tc,
separates two distinguishable Type-CE antiferromagnetic phases that are
metamagnetic. Measurements of the transport properties under hydrostatic
pressure were carried out on a compositions t a little below tc in order to
compare the effects of chemical vs. hydrostatic pressure on the phases that
compete with one another near t=tc.Comment: 10 pages. To be publised in Phys. Rev.
Improved high-temperature expansion and critical equation of state of three-dimensional Ising-like systems
High-temperature series are computed for a generalized Ising model with
arbitrary potential. Two specific ``improved'' potentials (suppressing leading
scaling corrections) are selected by Monte Carlo computation. Critical
exponents are extracted from high-temperature series specialized to improved
potentials, achieving high accuracy; our best estimates are:
, , , ,
. By the same technique, the coefficients of the small-field
expansion for the effective potential (Helmholtz free energy) are computed.
These results are applied to the construction of parametric representations of
the critical equation of state. A systematic approximation scheme, based on a
global stationarity condition, is introduced (the lowest-order approximation
reproduces the linear parametric model). This scheme is used for an accurate
determination of universal ratios of amplitudes. A comparison with other
theoretical and experimental determinations of universal quantities is
presented.Comment: 65 pages, 1 figure, revtex. New Monte Carlo data by Hasenbusch
enabled us to improve the determination of the critical exponents and of the
equation of state. The discussion of several topics was improved and the
bibliography was update
Ising Universality in Three Dimensions: A Monte Carlo Study
We investigate three Ising models on the simple cubic lattice by means of
Monte Carlo methods and finite-size scaling. These models are the spin-1/2
Ising model with nearest-neighbor interactions, a spin-1/2 model with
nearest-neighbor and third-neighbor interactions, and a spin-1 model with
nearest-neighbor interactions. The results are in accurate agreement with the
hypothesis of universality. Analysis of the finite-size scaling behavior
reveals corrections beyond those caused by the leading irrelevant scaling
field. We find that the correction-to-scaling amplitudes are strongly dependent
on the introduction of further-neighbor interactions or a third spin state. In
a spin-1 Ising model, these corrections appear to be very small. This is very
helpful for the determination of the universal constants of the Ising model.
The renormalization exponents of the Ising model are determined as y_t = 1.587
(2), y_h = 2.4815 (15) and y_i = -0.82 (6). The universal ratio Q =
^2/ is equal to 0.6233 (4) for periodic systems with cubic symmetry.
The critical point of the nearest-neighbor spin-1/2 model is K_c=0.2216546
(10).Comment: 25 pages, uuencoded compressed PostScript file (to appear in Journal
of Physics A
Suppression of charge-ordering and appearance of magnetoresistance in a spin-cluster glass manganite La0.3Ca0.7Mn0.8Cr0.2O3
The magnetic properties of electron-doped manganite La0.3Ca0.7MnO3 and
La0.3Ca0.7Mn0.8Cr0.2O3 polycrystalline samples prepared by sol-gel technique
have been investigated between 5 and 300 K in magnetic fields ranging from 0 to
5 T. The transition at 260 K, attributed to charge ordering in La0.3Ca0.7MnO3,
is completely suppressed in the Cr-substituted sample while the onset of a
magnetic remanence followed by the appearance of a magnetic irreversibility at
lower temperatures is observed in both samples. These features indicate that
ferromagnetic clusters coexist with either an antiferromagnetic phase for
La0.3Ca0.7MnO3 or a spin-cluster glass phase for La0.3Ca0.7Mn0.8Cr0.2O3 at the
lowest temperatures. The exponential temperature dependence of the resistivity
for the Cr-substituted sample is consistent with the small polaron hopping
model for 120 K < T < 300 K, while the data are better described by Mott's
hopping mechanism for T < 120 K. Whereas the parent compound La0.3Ca0.7MnO3 is
known to show no magnetoresistance, a large negative magnetoresistance is
observed in the La0.3Ca0.7Mn0.8Cr0.2O3 sample below 120 K. The appearance of
the CMR is attributed to spin dependent hopping between spin clusters and/or
between ferromagnetic domains
Spintronics: Fundamentals and applications
Spintronics, or spin electronics, involves the study of active control and
manipulation of spin degrees of freedom in solid-state systems. This article
reviews the current status of this subject, including both recent advances and
well-established results. The primary focus is on the basic physical principles
underlying the generation of carrier spin polarization, spin dynamics, and
spin-polarized transport in semiconductors and metals. Spin transport differs
from charge transport in that spin is a nonconserved quantity in solids due to
spin-orbit and hyperfine coupling. The authors discuss in detail spin
decoherence mechanisms in metals and semiconductors. Various theories of spin
injection and spin-polarized transport are applied to hybrid structures
relevant to spin-based devices and fundamental studies of materials properties.
Experimental work is reviewed with the emphasis on projected applications, in
which external electric and magnetic fields and illumination by light will be
used to control spin and charge dynamics to create new functionalities not
feasible or ineffective with conventional electronics.Comment: invited review, 36 figures, 900+ references; minor stylistic changes
from the published versio
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